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- Publisher
- Wiley
- Copyright
- Copyright © 2015 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim
- ISSN
- 1614-6832
- eISSN
- 1614-6840
- DOI
- 10.1002/aenm.201400812
- Publisher site
- See Article on Publisher Site
Abstract
The remarkably high open‐circuit voltage of methylammonium lead iodide perovskite solar cells is investigated. Both the theoretical maximum and the real open‐circuit voltage are predicted from electroluminescence and photovoltaic external quantum efficiency spectra. Radiative and non‐radiative recombination are quantified, where a source of non‐radiative recombination is found in the mesoscopic structure, independent of the Al2O3 or TiO2 scaffold. Without a hole‐transport layer, non‐radiative recombination is strongly enhanced, which reduces the open‐circuit voltage.
Journal
Advanced Energy Materials – Wiley
Published: Feb 1, 2015