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- Publisher
- Wiley
- Copyright
- © 2017 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim
- ISSN
- 1614-6832
- eISSN
- 1614-6840
- DOI
- 10.1002/aenm.201700561
- Publisher site
- See Article on Publisher Site
Abstract
A reversible room‐temperature aluminum–sulfur (Al‐S) battery is demonstrated with a strategically designed cathode structure and an ionic liquid electrolyte. Discharge–charge mechanism of the Al‐S battery is proposed based on a sequence of electrochemical, microscopic, and spectroscopic analyses. The electrochemical process of the Al‐S battery involves the formation of a series of polysulfides and sulfide. The high‐order polysulfides (Sx2−, x ≥ 6) are soluble in the ionic liquid electrolyte. Electrochemical transitions between S62− and the insoluble low‐order polysulfides or sulfide (Sx2−, 1 ≤ x < 6) are reversible. A single‐wall carbon nanotube coating applied to the battery separator helps alleviate the diffusion of the polysulfide species and reduces the polarization behavior of the Al‐S batteries.
Journal
Advanced Energy Materials – Wiley
Published: Sep 1, 2017
Keywords: ; ; ; ;