Access the full text.
Sign up today, get DeepDyve free for 14 days.
Lizhi Jiang, Kunlong Liu, Sung-Fu Hung, Lingyun Zhou, R. Qin, Qinghua Zhang, Pengxin Liu, L. Gu, Hao Chen, G. Fu, N. Zheng (2020)
Facet engineering accelerates spillover hydrogenation on highly diluted metal nanocatalystsNature Nanotechnology, 15
Xiaopeng Han, Guowei He, Yu He, Jinfeng Zhang, Xuerong Zheng, Lanlan Li, C. Zhong, Wenbin Hu, Yida Deng, Tianyi Ma (2018)
Engineering Catalytic Active Sites on Cobalt Oxide Surface for Enhanced Oxygen ElectrocatalysisAdvanced Energy Materials, 8
R. Lin, Jiawei Wan, Yu Xiong, Konglin Wu, W. Cheong, Gang Zhou, Dingsheng Wang, Q. Peng, Chen Chen, Yadong Li (2018)
Quantitative Study of Charge Carrier Dynamics in Well-Defined WO3 Nanowires and Nanosheets: Insight into the Crystal Facet Effect in Photocatalysis.Journal of the American Chemical Society, 140 29
Q. Pang, Dipan Kundu, M. Cuisinier, L. Nazar (2014)
Surface-enhanced redox chemistry of polysulphides on a metallic and polar host for lithium-sulphur batteriesNature Communications, 5
Xue Liu, Jiaqi Huang, Qiang Zhang, L. Mai (2017)
Nanostructured Metal Oxides and Sulfides for Lithium–Sulfur BatteriesAdvanced Materials, 29
Song Bai, Lili Wang, Zhengquan Li, Y. Xiong (2016)
Facet‐Engineered Surface and Interface Design of Photocatalytic MaterialsAdvanced Science, 4
Xiguang Han, Liang Li, Chao Wang (2012)
Synthesis of tin dioxide nanooctahedra with exposed high-index {332} facets and enhanced selective gas sensing properties.Chemistry, an Asian journal, 7 7
Jianbin Zhou, Xiaojing Liu, Linqin Zhu, Jie Zhou, Yong Guan, Liang Chen, Shuwen Niu, Jinyan Cai, Da-Wen Sun, Yongchun Zhu, Jin Du, Gongming Wang, Yitai Qian (2018)
Deciphering the Modulation Essence of p Bands in Co-Based Compounds on Li-S ChemistryJoule
A. Manthiram, Yongzhu Fu, Sheng‐Heng Chung, Chenxi Zu, Yu‐Sheng Su (2014)
Rechargeable lithium-sulfur batteries.Chemical reviews, 114 23
Weijiang Xue, Zhe Shi, Liumin Suo, Chao Wang, Ziqiang Wang, Haozhe Wang, K. So, Andrea Maurano, Daiwei Yu, Yuming Chen, Long Qie, Zhi Zhu, Guiyin Xu, J. Kong, Ju Li (2019)
Intercalation-conversion hybrid cathodes enabling Li–S full-cell architectures with jointly superior gravimetric and volumetric energy densitiesNature Energy, 4
Tingting Sun, Xiaomei Zhao, Bo Li, H. Shu, Lipan Luo, Wenlong Xia, Manfang Chen, P. Zeng, Xiukang Yang, P. Gao, Yong Pei, Xian-you Wang (2021)
NiMoO4 Nanosheets Anchored on NS Doped Carbon Clothes with Hierarchical Structure as a Bidirectional Catalyst toward Accelerating Polysulfides Conversion for LiS BatteryAdvanced Functional Materials, 31
Cheng Zheng, Shuzhang Niu, Wei Lv, Guangmin Zhou, Jia Li, Shaoxun Fan, Yaqian Deng, Zheng‐Ze Pan, Baohua Li, F. Kang, Quan-hong Yang (2017)
Propelling polysulfides transformation for high-rate and long-life lithium–sulfur batteriesNano Energy, 33
Xin Wang, Dan Luo, Jiayi Wang, Zhenghao Sun, G. Cui, Yuxuan Chen, Tong Wang, Lirong Zheng, Yan Zhao, L. Shui, Guofu Zhou, K. Kempa, Yongguang Zhang, Zhongwei Chen (2021)
Strain Engineering of a MXene/CNT Hierarchical Porous Hollow Microsphere Electrocatalyst for a High-Efficiency Lithium Polysulfide Conversion Process.Angewandte Chemie
L. Lv, C. Guo, Weiwei Sun, Yong Wang (2018)
Strong Surface-Bound Sulfur in Carbon Nanotube Bridged Hierarchical Mo2 C-Based MXene Nanosheets for Lithium-Sulfur Batteries.Small, 15 3
Shaopeng Rong, Pengyi Zhang, Fang Liu, Yajie Yang (2018)
Engineering Crystal Facet of α-MnO2 Nanowire for Highly Efficient Catalytic Oxidation of Carcinogenic Airborne FormaldehydeACS Catalysis, 8
Zixiong Shi, Matthew Li, Jingyu Sun, Zhongwei Chen (2021)
Defect Engineering for Expediting Li–S Chemistry: Strategies, Mechanisms, and PerspectivesAdvanced Energy Materials, 11
Na Tian, Zhiyou Zhou, Shigang Sun, Yong Ding, Zhong Wang (2007)
Synthesis of Tetrahexahedral Platinum Nanocrystals with High-Index Facets and High Electro-Oxidation ActivityScience, 316
Ruo Wang, C. Luo, Tianshuai Wang, Guangmin Zhou, Yaqian Deng, Yan‐Bing He, Qianfan Zhang, F. Kang, Wei Lv, Quan-hong Yang (2020)
Bidirectional Catalysts for Liquid–Solid Redox Conversion in Lithium–Sulfur BatteriesAdvanced Materials, 32
Zhen Li, Jintao Zhang, B. Guan, Da Wang, Li‐Min Liu, X. Lou (2016)
A sulfur host based on titanium monoxide@carbon hollow spheres for advanced lithium–sulfur batteriesNature Communications, 7
Huan Zhao, Dan Zhang, Hongdong Li, Wenjing Qi, Xueke Wu, Yi Han, Wenwen Cai, Zuochao Wang, J. Lai, Lei Wang (2020)
Exposure of Definite Palladium Facets Boosts Electrocatalytic Nitrogen Fixation at Low OverpotentialAdvanced Energy Materials, 10
Lei Wang, N. Nguyen, Zhiqiang Shen, P. Schmuki, Yingpu Bi (2018)
Hematite dodecahedron crystals with high-index facets grown and grafted on one dimensional structures for efficient photoelectrochemical H2 generationNano Energy
Fulai Qi, Zhenhua Sun, Xia-Lu Fan, Zhenxing Wang, Ying Shi, Guangjian Hu, Feng Li (2021)
Tunable Interaction between Metal‐Organic Frameworks and Electroactive Components in Lithium–Sulfur Batteries: Status and PerspectivesAdvanced Energy Materials, 11
Xiaoqing Huang, Zipeng Zhao, Jing-min Fan, Y. Tan, N. Zheng (2011)
Amine-assisted synthesis of concave polyhedral platinum nanocrystals having {411} high-index facets.Journal of the American Chemical Society, 133 13
Y. Zhong, L. Yin, P. He, W. Liu, Zishan Wu, Hailiang Wang (2018)
Surface Chemistry in Cobalt Phosphide-Stabilized Lithium-Sulfur Batteries.Journal of the American Chemical Society, 140 4
Y. Qiu, Lishuang Fan, Maoxu Wang, X. Yin, Xian Wu, Xun Sun, Da Tian, Bin Guan, D. Tang, Naiqing Zhang (2020)
Precise Synthesis of Fe-N2 Sites with High Activity and Stability for Long-Life Lithium-Sulfur Batteries.ACS nano
Ya‐Tao Liu, Dian‐Dian Han, Lu Wang, Guoran Li, Shengqi Liu, Xueping Gao (2019)
NiCo2O4 Nanofibers as Carbon‐Free Sulfur Immobilizer to Fabricate Sulfur‐Based Composite with High Volumetric Capacity for Lithium–Sulfur BatteryAdvanced Energy Materials, 9
Zhengqing Ye, Ying Jiang, Li Li, Feng Wu, Renjie Chen (2020)
A High‐Efficiency CoSe Electrocatalyst with Hierarchical Porous Polyhedron Nanoarchitecture for Accelerating Polysulfides Conversion in Li–S BatteriesAdvanced Materials, 32
Lele Peng, Ziyang Wei, Chengzhang Wan, Jing Li, Zhuo Chen, Da-Ming Zhu, D. Baumann, Haotian Liu, C. Allen, Xiang Xu, A. Kirkland, I. Shakir, Z. Almutairi, S. Tolbert, B. Dunn, Yu Huang, P. Sautet, X. Duan (2020)
A fundamental look at electrocatalytic sulfur reduction reactionNature Catalysis, 3
Guangmin Zhou, Hongzhen Tian, Yang Jin, X. Tao, Bofei Liu, Rufan Zhang, Z. Seh, Denys Zhuo, Yayuan Liu, Jie Sun, Jie Zhao, Chenxi Zu, David Wu, Qianfan Zhang, Yi Cui (2017)
Catalytic oxidation of Li2S on the surface of metal sulfides for Li−S batteriesProceedings of the National Academy of Sciences, 114
Xiaoxia Chen, Suyuan Zeng, Haliya Muheiyati, Yanjun Zhai, Chuanchuan Li, Xuyang Ding, Lu Wang, Debao Wang, Liqiang Xu, Yanyan He, Yitai Qian (2019)
Double-Shelled Ni–Fe–P/N-Doped Carbon Nanobox Derived from a Prussian Blue Analogue as an Electrode Material for K-Ion Batteries and Li–S BatteriesACS Energy Letters
Hao Wu, Tong Yang, Yonghua Du, Lei Shen, G. Ho (2018)
Identification of Facet‐Governing Reactivity in Hematite for Oxygen EvolutionAdvanced Materials, 30
Yi Chen, Tianyi Wang, Huajun Tian, D. Su, Qiang Zhang, Guoxiu Wang (2021)
Advances in Lithium–Sulfur Batteries: From Academic Research to Commercial ViabilityAdvanced Materials, 33
Chen Zhao, Gui‐Liang Xu, Zhou Yu, Leicheng Zhang, In-hui Hwang, Yudi Mo, Yuxun Ren, Lei Cheng, Cheng-Jun Sun, Yang Ren, X. Zuo, Jun-tao Li, Shigang Sun, K. Amine, T. Zhao (2020)
A high-energy and long-cycling lithium–sulfur pouch cell via a macroporous catalytic cathode with double-end binding sitesNature Nanotechnology, 16
Jiarui He, A. Manthiram (2019)
Long‐Life, High‐Rate Lithium–Sulfur Cells with a Carbon‐Free VN Host as an Efficient Polysulfide Adsorbent and Lithium Dendrite InhibitorAdvanced Energy Materials, 10
E. Salhabi, Jilu Zhao, Jiangyan Wang, Mei Yang, Bao Wang, Dan Wang (2019)
Hollow Multi-Shelled Structural TiO2-x with Multiple Spatial Confinement for Long-Life Lithium-Sulfur Batteries.Angewandte Chemie
Xiguang Han, Mingshang Jin, Shuifen Xie, Q. Kuang, Zhiyuan Jiang, Yaqi Jiang, Zhaoxiong Xie, Lan-Sun Zheng (2009)
Synthesis of tin dioxide octahedral nanoparticles with exposed high-energy {221} facets and enhanced gas-sensing properties.Angewandte Chemie, 48 48
Xia Huang, Jiayong Tang, Bin Luo, R. Knibbe, Tongen Lin, Han Hu, M. Rana, Yuxiang Hu, Xiao-bo Zhu, Q. Gu, Dan Wang, Lianzhou Wang (2019)
Sandwich‐Like Ultrathin TiS2 Nanosheets Confined within N, S Codoped Porous Carbon as an Effective Polysulfide Promoter in Lithium‐Sulfur BatteriesAdvanced Energy Materials, 9
Yu Yao, Haiyun Wang, Hai Yang, Sifan Zeng, Rui Xu, Fanfan Liu, Pengcheng Shi, Yuezhan Feng, Kai Wang, Wenjin Yang, Xiaojun Wu, Wei Luo, Yan Yu (2019)
A Dual‐Functional Conductive Framework Embedded with TiN‐VN Heterostructures for Highly Efficient Polysulfide and Lithium Regulation toward Stable Li–S Full BatteriesAdvanced Materials, 32
Maoxu Wang, Lishuang Fan, Xun Sun, Bin Guan, Bo Jiang, Xian Wu, Da Tian, Kening Sun, Y. Qiu, X. Yin, Yu Zhang, Naiqing Zhang (2020)
Nitrogen-Doped CoSe2 as a Bifunctional Catalyst for High Areal Capacity and Lean Electrolyte of Li–S BatteryACS energy letters, 5
Y. Jiao, Yao Zheng, K. Davey, S. Qiao (2016)
Activity origin and catalyst design principles for electrocatalytic hydrogen evolution on heteroatom-doped grapheneNature Energy, 1
Chao Ye, Y. Jiao, Huanyu Jin, A. Slattery, K. Davey, Haihui Wang, S. Qiao (2018)
2D MoN-VN Heterostructure To Regulate Polysulfides for Highly Efficient Lithium-Sulfur Batteries.Angewandte Chemie, 57 51
Yongguang Zhang, Gaoran Li, Jiayi Wang, G. Cui, Xiaoling Wei, L. Shui, K. Kempa, Guofu Zhou, Xin Wang, Zhongwei Chen (2020)
Hierarchical Defective Fe3‐xC@C Hollow Microsphere Enables Fast and Long‐Lasting Lithium–Sulfur BatteriesAdvanced Functional Materials, 30
Zihan Shen, Mengqiu Cao, Zili Zhang, J. Pu, Chenglin Zhong, Jiachen Li, Hai-xia Ma, Fujun Li, Jia Zhu, F. Pan, Huigang Zhang (2019)
Efficient Ni2Co4P3 Nanowires Catalysts Enhance Ultrahigh‐Loading Lithium–Sulfur Conversion in a Microreactor‐Like BatteryAdvanced Functional Materials, 30
Jungjin Park, Byeong-Chul Yu, J. Park, J. Choi, Chunjoong Kim, Y. Sung, J. Goodenough (2017)
Tungsten Disulfide Catalysts Supported on a Carbon Cloth Interlayer for High Performance Li–S BatteryAdvanced Energy Materials, 7
Liang-Liang Feng, Guangtao Yu, Yuanyuan Wu, Guodong Li, Hui Li, Yuanhui Sun, Tewodros Asefa, Wei Chen, Xiaoxin Zou (2015)
High-index faceted Ni3S2 nanosheet arrays as highly active and ultrastable electrocatalysts for water splitting.Journal of the American Chemical Society, 137 44
Jinping Zhao, S. Pei, W. Ren, Libo Gao, Hui‐Ming Cheng (2010)
Efficient preparation of large-area graphene oxide sheets for transparent conductive films.ACS nano, 4 9
Songwei Gao, Nü Wang, Shuai Li, Dianming Li, Zhimin Cui, G. Yue, Jingchong Liu, Xiaoxian Zhao, Lei Jiang, Yong Zhao (2019)
Multi-wall Sn/SnO2@Carbon Hollow Nanofibers Anode Material for High-Rate and Long-Life Lithium-Ion Batteries.Angewandte Chemie
Xue Wang, Xiguang Han, Shuifen Xie, Q. Kuang, Yaqi Jiang, Subing Zhang, Xiaoliang Mu, Guangxu Chen, Zhaoxiong Xie, Lan-Sun Zheng (2012)
Controlled synthesis and enhanced catalytic and gas-sensing properties of tin dioxide nanoparticles with exposed high-energy facets.Chemistry, 18 8
Dan Luo, Gaoran Li, Ya-Ping Deng, Zhen Zhang, Jingde Li, Ruilin Liang, Matthew Li, Yi Jiang, Weiwei Zhang, Yangshuai Liu, W. Lei, A. Yu, Zhongwei Chen (2019)
Synergistic Engineering of Defects and Architecture in Binary Metal Chalcogenide toward Fast and Reliable Lithium–Sulfur BatteriesAdvanced Energy Materials, 9
Jiadong Shen, Xijun Xu, Jun Liu, Zhengbo Liu, Fangkun Li, R. Hu, Jiangwen Liu, Xianhua Hou, Yuezhan Feng, Yan Yu, Min Zhu (2019)
Mechanistic Understanding of Metal Phosphide Host for Sulfur Cathode in High-Energy-Density Lithium-Sulfur Batteries.ACS nano
Xiao Liang, Connor Hart, Q. Pang, A. Garsuch, T. Weiss, L. Nazar (2015)
A highly efficient polysulfide mediator for lithium–sulfur batteriesNature Communications, 6
Chi Xiao, Bang-An Lu, Pengchong Xue, Na Tian, Zhiyou Zhou, Xiao Lin, Wen-Feng Lin, Shigang Sun (2020)
High-Index-Facet- and High-Surface-Energy Nanocrystals of Metals and Metal Oxides as Highly Efficient CatalystsJoule, 4
Zhenzhen Du, Xingjia Chen, Wei Hu, Chenghao Chuang, Shuai-Lei Xie, Ajuan Hu, Wensheng Yan, X. Kong, Xiaojun Wu, Hengxing Ji, L. Wan (2019)
Cobalt in Nitrogen-Doped Graphene as Single-Atom Catalyst for High-Sulfur Content Lithium-Sulfur Batteries.Journal of the American Chemical Society, 141 9
Zhe Yuan, Hong‐Jie Peng, Tingzheng Hou, Jiaqi Huang, Chengmeng Chen, Dai‐Wei Wang, Xin‐Bing Cheng, F. Wei, Qiang Zhang (2016)
Powering Lithium-Sulfur Battery Performance by Propelling Polysulfide Redox at Sulfiphilic Hosts.Nano letters, 16 1
Hong Yuan, Hong‐Jie Peng, Bo‐Quan Li, Jin Xie, Long Kong, Mengqiang Zhao, Xiao Chen, Jiaqi Huang, Qiang Zhang (2018)
Conductive and Catalytic Triple‐Phase Interfaces Enabling Uniform Nucleation in High‐Rate Lithium–Sulfur BatteriesAdvanced Energy Materials, 9
Da Tian, Xueqin Song, Maoxu Wang, Xian Wu, Y. Qiu, Bin Guan, Xianzhu Xu, Lishuang Fan, Naiqing Zhang, Kening Sun (2019)
MoN Supported on Graphene as a Bifunctional Interlayer for Advanced Li‐S BatteriesAdvanced Energy Materials, 9
Lei Zhou, Lei Zhou, D. Danilov, D. Danilov, R. Eichel, R. Eichel, P. Notten, P. Notten, P. Notten (2020)
Host Materials Anchoring Polysulfides in Li–S Batteries ReviewedAdvanced Energy Materials, 11
Controlling exposed crystal facets through crystal facet engineering is an efficient strategy for enhancing the catalytic activity of nanocrystalline catalysts. Herein, the active tin dioxide nano–octahedra enclosed by {332} crystal facets (SnO2 {332}) are synthesized on reduced graphene oxide and demonstrate powerful chemisorption and catalytic ability, accelerating the redox kinetics of sulfur species in lithium–sulfur chemistry. Attributed to abundant unsaturated–coordinated Sn sites on {332} crystal planes, SnO2 {332} has outstanding adsorption and catalytic properties. The material not only adsorbs and converts polysulfides efficiently, but also prominently lowers the decomposition energy barrier of Li2S. The batteries with these high active electrocatalysts exhibit excellent cycling stability with a low capacity attenuation of 0.021% every cycle during 2000 cycles at 2 C. Even with a sulfur loading of 8.12 mg cm−2, the batteries can still cycle stably and maintain a prominent areal capacity of 6.93 mAh cm−2 over 100 cycles. This research confirms that crystal facet engineering is a promising strategy to optimize the performance of catalysts, deepens the understanding of surface structure‐oriented electrocatalysis in Li–S chemistry, while aiding the rational design of advanced sulfur electrodes.
Advanced Energy Materials – Wiley
Published: Dec 1, 2021
Keywords: crystal facet engineering; electrocatalysis; Li–S batteries; redox kinetics; SnO 2 nanocrystals
Read and print from thousands of top scholarly journals.
Already have an account? Log in
Bookmark this article. You can see your Bookmarks on your DeepDyve Library.
To save an article, log in first, or sign up for a DeepDyve account if you don’t already have one.
Copy and paste the desired citation format or use the link below to download a file formatted for EndNote
Access the full text.
Sign up today, get DeepDyve free for 14 days.
All DeepDyve websites use cookies to improve your online experience. They were placed on your computer when you launched this website. You can change your cookie settings through your browser.