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中 国 化 学 Concise Reports Radical Heteroarylalkylation of Alkenes via Three-Component Docking-Migration Thio- etherification Cascade A novel, rational-designed approach to access various heteroaryl-substituted alkyl thioethers was developed via docking-migration cascade process. By utilizing three components involving alkene, dual-function reagent, and thioetherificating reagent, radical heteroarylalkylation of alkenes fol- lowed by thiolation of the alkyl radical intermediates proceeded smoothly, manifesting well com- patibility of substrates and cascade transformations. Furthermore, this protocol also features mild Tao Niu, Jige Liu, Xinxin Wu, Chen Zhu* conditions, broad substrate scope, and wide product diversity. Sequential Ir-Catalyzed Allylation/2-aza-Cope Rearrangement Strategy for the Construction of Chiral Homoallylic Amines Sequential Ir-catalyzed asymmetric allylation/2-aza-Cope rearrangement of arylidene ami- no-malonates with allylic carbonates was successfully developed, and a variety of enantioenriched homoallylic amine derivatives were obtained in high yields with good chirality transfer and excel- Ruo-Qing Wang, Chong Shen, Xiang Cheng, lent E/Z-geometry control (up to 99% yield, 96% ee). Compared with previous dual catalytic system Zuo-Fei Wang, Hai-Yan Tao, Xiu-Qin Dong,* established for this transformation, the current mono metal catalytic system provides a simpler Chun-Jiang Wang* and more practical protocol employing the readily available starting materials. Structurally Interesting Diarymethane Deriva- tives from Securidaca inappendiculata Bin Zhou, Yan Wu,
Chinese Journal of Chemistry – Wiley
Published: Aug 1, 2020
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