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- Publisher
- Wiley
- Copyright
- © 2021 Wiley‐VCH GmbH
- ISSN
- 1614-6832
- eISSN
- 1614-6840
- DOI
- 10.1002/aenm.202101928
- Publisher site
- See Article on Publisher Site
Abstract
Potassium ion battery (PIB) is a potential candidate for future large‐scale energy storage. A key challenge is that the (de)potassiation stability of graphitic carbon anodes is hampered by the limited (002) interlayer spacing. Amorphous carbon with a hierarchical structure can buffer the volume change during repeated (de)potassiation and enable stable cycling. Herein, a direct pyrolysis approach is demonstrated to synthesize a highly nitrogen‐doped (26.7 at.%) accordion‐like carbon anode composed of thin carbon nanosheets and a turbostratic crystalline structure. The hierarchical structure of accordion‐like carbon is endowed by a self‐assembly process during pyrolysis carbonization. The hierarchical nitrogen‐doped accordion structure enables a high reversible capacity of 346 mAh g−1 and superior cycling stability. This work constitutes a general synthesis methodology that can be used to prepare hierarchical carbon anodes for advanced PIBs.
Journal
Advanced Energy Materials – Wiley
Published: Nov 1, 2021
Keywords: edge nitrogen dopant; nitrogen‐doped carbon; potassium ion batteries; pyrolysis; self‐assembly