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- Publisher
- Wiley
- Copyright
- © 2020 Wiley‐VCH GmbH
- eISSN
- 2192-6506
- DOI
- 10.1002/cplu.202000618
- Publisher site
- See Article on Publisher Site
Abstract
The quality of ion‐selective membranes determines the efficiency of Vanadium Flow Batteries (VFBs), and alternatives to expensive Nafion™ materials are actively being searched for. One of the membrane architecture approaches is to imitate the Nafion™ structure with two separate phases: a conductive sulfonated polymer and an inner matrix. We introduce a new composite material based on sulfonated styrene polymerized inside the pores of a stretched PTFE matrix. Variation of polystyrene content and a sulfonation degree allowed to obtain membranes with IEC from to 0.96 to 1.84 mmol/g. Balanced vanadium permeability (ca. 5.5 ⋅ 10−6 cm2/min) and proton conductivity (ca. 50 mS/cm) were achieved for the material with 21–23 % polystyrene content and a sulfonation degree up to 94 %. Membranes showed stable cycling with 81 % energy efficiency in a single‐cell VFB. This work contributes to the existing knowledge of Nafion alternatives by providing a cheap and scalable method of membrane production.
Journal
ChemPlusChem – Wiley
Published: Dec 1, 2020
Keywords: ; ; ; ;