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- Publisher
- Springer Journals
- Copyright
- Copyright © 2018 by Springer-Verlag GmbH Germany, part of Springer Nature
- Subject
- Chemistry; Electrochemistry; Renewable and Green Energy; Optical and Electronic Materials; Condensed Matter Physics; Energy Storage
- ISSN
- 0947-7047
- eISSN
- 1862-0760
- DOI
- 10.1007/s11581-018-2754-5
- Publisher site
- See Article on Publisher Site
Abstract
The layered structure of LiNi1/3Mn1/3Co1/3 – x Y x O2 with different concentration of yttrium substituted (x = 0.00, 0.01, 0.03, and 0.05) cathode material was synthesized using the sol-gel method, followed by high-temperature calcination process. The influence of Y substitution on the microstructure and electrochemical performances of the prepared materials were investigated using X-ray diffraction (XRD), transmission electron microscopy (TEM), cyclic voltammetry and galvanostatic charge/discharge test respectively. The XRD result showed that the LiNi1/3Mn1/3Co1/3 − x Y x O2 has a well-ordered hexagonal α-NaFeO2 structure with high crystallinity. The surface morphology of pristine material and Y-doped electrode material revealed the spherical-shaped particles which are uniformly distributed. The cyclic voltammograms of the proposed cathode material also yield a well-defined redox peaks at their corresponding potentials. As the doping of yttrium increases, the discharge capacity also increases attributed to the superior capacity retention at high voltage (4.2 V) even after 100 cycles. Therefore, this composition is a promising cathode material for lithium-ion batteries.
Journal
Ionics – Springer Journals
Published: Oct 16, 2018