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The preparation of nanostructured anode materials which can adapt to lithiation strain with higher structural stability and specific capacity is the primary challenge for the development of lithium-ion batteries (LIBs). Herein, we developed a carbon-coated, fluorine-molybdenum-doped SnO2 (SnO2@C-MoF4) green composite with high long-term cycling stability and specific capacity. The composite materials were prepared by the NaCl template method. The carbonaceous composites prepared by the NaCl template method will form a three-dimensional (3D) interconnected carbon structure, which can well alleviate the problem of the large volume change of SnO2 during the lithium intercalation/delithiation process. Thereby, under the premise of maintaining a higher specific capacity, it can improve the long-term cycling stability of tin-based lithium-ion battery anode materials to meet the requirements of high-performance lithium-ion battery anode materials. The SnO2@C-MoF4 composites prepared by the template method have an outstanding specific capacity (845.10 mAh/g) at 0.2 A/g, and superior cycling stability (749.19 mAh/g) was obtained after 800 charge–discharge cycles at 1.0 A/g.
Ionics – Springer Journals
Published: Oct 1, 2022
Keywords: Lithium-ion battery; Anode; NaCl; 3D interconnected carbon network; SnO2
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