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- Publisher
- Springer Journals
- Copyright
- Copyright © Higher Education Press 2021
- ISSN
- 2095-1701
- eISSN
- 2095-1698
- DOI
- 10.1007/s11708-021-0750-3
- Publisher site
- See Article on Publisher Site
Abstract
An environment-friendly, water-soluble, and cellulose based binder (lithium carboxymethyl cellulose, CMC-Li) was successfully synthesized by using Li+ to replace Na+ in the commercial sodium carboxymethyl cellulose (CMC-Na). Li-O2 batteries based on the CMC-Li binder present enhanced discharge specific capacities (11151 mAh/g at 100 mA/g) and a superior cycling stability (100 cycles at 200 mA/g) compared with those based on the CMC-Na binder. The enhanced performance may originate from the electrochemical stability of the CMC-Li binder and the ion-conductive nature of CMC-Li, which promotes the diffusion of Li+ in the cathode and consequently retards the increase of charge transfer resistance of the cathode during cycling. The results show that the water-soluble CMC-Li binder can be a green substitute for poly(vinylidene fluoride) (PVDF) binder based on organic solvent in the lithium oxygen batteries (LOBs).
Journal
Frontiers in Energy – Springer Journals
Published: Jun 1, 2022
Keywords: cellulose; binder; specific capacity; cyclability; lithium-oxygen batteries