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Electrocaloric behavior and temperature dependent scaling of dynamic hysteresis of BaxSr1-xTiO3 (x = 0.7, 0.8 and 0.9) bulk ceramics

Electrocaloric behavior and temperature dependent scaling of dynamic hysteresis of BaxSr1-xTiO3... This article presents electrocaloric effect in BaxSr1-xTiO3 ferroelectric ceramics using an indirect approach based on Maxwell’s relations. The peak electrocaloric performance is found to be an adiabatic temperature change of 0.67, 0.83, and 0.61 K and isothermal entropy change of 0.9, 1, and 0.7 J/kg.K for x = 0.7, 0.8, and 0.9, respectively, under an electric field of 33 kV/cm. The electrocaloric coefficient of performance (COP) of materials were also estimated as 17, 5.47, and 5.68 when x = 0.7, 0.8, and 0.9, respectively, in BaxSr1-xTiO3 at 33 kV/cm (303 K). Further, the ferroelectric hysteresis parameters scaling relations of coercive field (E c) and remnant polarization (P r) as a function of temperature have been estimated. The back switching polarization (P bc) as a function of temperature (T) was estimated by the Arrhenius law in order to understand the domain dynamics, and the average activation energy was evaluated. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Journal of the Australian Ceramic Society Springer Journals

Electrocaloric behavior and temperature dependent scaling of dynamic hysteresis of BaxSr1-xTiO3 (x = 0.7, 0.8 and 0.9) bulk ceramics

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Publisher
Springer Journals
Copyright
Copyright © 2017 by Australian Ceramic Society
Subject
Materials Science; Ceramics, Glass, Composites, Natural Materials; Materials Engineering; Inorganic Chemistry
ISSN
2510-1560
eISSN
2510-1579
DOI
10.1007/s41779-017-0170-3
Publisher site
See Article on Publisher Site

Abstract

This article presents electrocaloric effect in BaxSr1-xTiO3 ferroelectric ceramics using an indirect approach based on Maxwell’s relations. The peak electrocaloric performance is found to be an adiabatic temperature change of 0.67, 0.83, and 0.61 K and isothermal entropy change of 0.9, 1, and 0.7 J/kg.K for x = 0.7, 0.8, and 0.9, respectively, under an electric field of 33 kV/cm. The electrocaloric coefficient of performance (COP) of materials were also estimated as 17, 5.47, and 5.68 when x = 0.7, 0.8, and 0.9, respectively, in BaxSr1-xTiO3 at 33 kV/cm (303 K). Further, the ferroelectric hysteresis parameters scaling relations of coercive field (E c) and remnant polarization (P r) as a function of temperature have been estimated. The back switching polarization (P bc) as a function of temperature (T) was estimated by the Arrhenius law in order to understand the domain dynamics, and the average activation energy was evaluated.

Journal

Journal of the Australian Ceramic SocietySpringer Journals

Published: Dec 27, 2017

References