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N.I. Kol'tsov (2021)
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N.I. Kol'tsov (2020)
10.1134/S0023158420030143Kinet. Catal, 61
An approach is developed to define conservation laws for the steady-state chemical reactions proceeding with arbitrary kinetics in an open isothermal reactor with longitudinal and radial diffusion of reactants (reactor with incomplete mixing, RIM). Dissipative structures that follow from the conservation laws, which describe the distribution of the complexes of reactant concentrations in the RIM as a function of the ratios between the reactant diffusion coefficients, are investigated. Examples of the definition and use of conservation laws and dissipative structures to solve the inverse problem of identifying the reaction mechanisms in an open RIM are given.
Kinetics and Catalysis – Springer Journals
Published: Nov 1, 2021
Keywords: chemical reactions; kinetic law; arbitrary kinetics; open reactor with incomplete mixing; conservation laws; dissipative structures; inverse problem
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