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Carbon dioxide utilization in methanol synthesis plant: process modeling

Carbon dioxide utilization in methanol synthesis plant: process modeling AbstractThe conversion of CO2 to methanol holds great promise, as it offers a pathway to reduce CO2 level in the atmosphere and also produce valuable components. In this study, a typical methanol synthesis plant for CO2 conversion was numerically modeled. Effect of fresh feed to plant parameters (i.e., pressure and CO2 concentration) as well as the influence of recycle ratio on the reactor performance was investigated. Hence, all essential equipment, including compressor, mixer, heat exchanger, reactor, and liquid–vapor separator were considered in the model. Then, at the best operating conditions, thermal behavior and components distribution along the length and radius of the reactor were predicted. Finally, the effect of inert gases was investigated in the methanol production process and the results were compared with the conventional route (CR), which uses natural gas for methanol synthesis. The results revealed that in the absence of inert gases and by employing a recycle stream in the process, CO2 hydrogenation leads to 13 ton/day production of methanol more than CR. While in the feedstock containing 20% inert gases, which is closer to the realistic case, methanol production rate is 45 ton/day lower than CR. These findings prospect a promising approach for the production of green methanol from carbon dioxide and hydrogen. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Chemical Product and Process Modeling de Gruyter

Carbon dioxide utilization in methanol synthesis plant: process modeling

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Publisher
de Gruyter
Copyright
© 2020 Walter de Gruyter GmbH, Berlin/Boston
ISSN
1934-2659
eISSN
1934-2659
DOI
10.1515/cppm-2020-0038
Publisher site
See Article on Publisher Site

Abstract

AbstractThe conversion of CO2 to methanol holds great promise, as it offers a pathway to reduce CO2 level in the atmosphere and also produce valuable components. In this study, a typical methanol synthesis plant for CO2 conversion was numerically modeled. Effect of fresh feed to plant parameters (i.e., pressure and CO2 concentration) as well as the influence of recycle ratio on the reactor performance was investigated. Hence, all essential equipment, including compressor, mixer, heat exchanger, reactor, and liquid–vapor separator were considered in the model. Then, at the best operating conditions, thermal behavior and components distribution along the length and radius of the reactor were predicted. Finally, the effect of inert gases was investigated in the methanol production process and the results were compared with the conventional route (CR), which uses natural gas for methanol synthesis. The results revealed that in the absence of inert gases and by employing a recycle stream in the process, CO2 hydrogenation leads to 13 ton/day production of methanol more than CR. While in the feedstock containing 20% inert gases, which is closer to the realistic case, methanol production rate is 45 ton/day lower than CR. These findings prospect a promising approach for the production of green methanol from carbon dioxide and hydrogen.

Journal

Chemical Product and Process Modelingde Gruyter

Published: Dec 13, 2021

Keywords: CO 2 hydrogenation; CO 2 utilization; methanol synthesis plant; two-dimensional model

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