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A new method of synthesis of functionally substituted benzaldehydes by catalytic debromometoxylation of dibromomethylarenes with benzaldehyde dimethyl acetal has been suggested. Anhydrous zinc chloride has been used as a catalyst. Being soft Lewis acid, it formed no strong complex with aldehyde...
Quantum-chemical calculations by the density functional theory method at the B3LYP/6- 311++G** level have shown that the fulvene form of pentamethoxycarbonylcyclopentadiene 1 in the gas phase is more favorable in energy than cyclopentadiene form 2 by ΔE
ZPE = 7.8 kcal/mol. The fluxional behavior...
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