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Imines are photoaddressable motifs useful in the development of new generations of molecular switches, but their operation with low‐energy photons and control over isomer stability remain challenging. Based on a computational design, we developed phenylimino indolinone (PIO), a...
We report herein the development of stereodivergent syntheses of enantioenriched homoallylic alcohols using chiral nonracemic α‐CH2Bpin‐substituted crotylboronate. Chiral phosphoric acid (S)‐A‐catalyzed asymmetric allyl addition with the reagent gave Z‐anti‐homoallylic alcohols with excellent...
By virtue of a fundamentally new reaction model of azomethine ylide serving as a two‐atom synthon, we present the first example of stereodivergent preparation of γ‐butyrolactones via synergistic Cu/Ir‐catalyzed asymmetric cascade allylation/lactonization, and all four stereoisomers of...
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