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A total synthesis of 17‐membered macrocyclolipopeptide dysoxylactam A, a potent agent reversing P‐glycoprotein (P‐gp)‐mediated multidrug resistance (MDR) in cancer cells, was developed from the starting material (S)‐2‐methylbutanal in a linear sequence of 12 steps with 23.2% overall yield. The...
New blue‐light promoted methods for the addition of iodoacetonitrile (ICH2CN) to alkene/alkynes have been developed. The reaction led to the formation of cyanoalkylated products when conjugated alkene/styrene was used. In the case of alkynes and non‐conjugated alkenes, iodoalkylation takes place...
Data‐driven approach has emerged as a powerful strategy in the construction of structure‐performance relationships in organic synthesis. To close the gap between mechanistic understanding and synthetic prediction, we have made efforts to implement mechanistic knowledge in machine learning...
Liquid fed fuel cells such as direct formic acid fuel cells (DFAFCs) are considered to be promising power sources for portable electronic devices. However, the poison of CO intermediates on the state‐of‐the‐art platinum and palladium‐based electrocatalysts for the formic acid oxidation reaction...
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